Search results for "Photon antibunching"
showing 8 items of 8 documents
Optical Microscopy and Spectroscopy of Single Molecules
2006
Photon antibunching in the optical near field
2010
International audience; We show that a combination of the field-susceptibility technique with the optical Bloch equations gives access to the temporal evolution of the populations and coherences of any quantum system placed in the optical near field of a nanostructure. In particular, we show that the near-field evanescent states, confined around dielectric or plasmonic particles, can be used to modify and control the photon statistics of the quantum system. This theoretical scheme leads to second-order autocorrelation functions in good agreement with recent experimental measurements performed with nitrogen-vacancy center in diamond nanocrystals placed in interaction with gold nanoparticles.
Acoustically driven photon antibunching in nanowires.
2011
The oscillating piezoelectric field of a surface acoustic wave (SAW) is employed to transport photoexcited carriers, as well as to spatially control exciton recombination in GaAs-based nanowires (NWs) on a subns time scale. The experiments are carried out in core-shell NWs transferred to a SAW delay line on a LiNbO(3) crystal. Carriers generated in the NW by a focused laser spot are acoustically transferred to a second location, leading to the remote emission of subns light pulses synchronized with the SAW phase. The dynamics of the carrier transport, investigated using spatially and time-resolved photoluminescence, is well-reproduced by computer simulations. The high-frequency contactless …
Single photon emission from impurity centers in AlGaAs epilayers on Ge and Si substrates
2012
We show that the epitaxial growth of thin layers of AlGaAs on Ge and Si substrates allows to obtain single photon sources by exploiting the sparse and unintentional contamination with acceptors of the AlGaAs. Very bright and sharp single photoluminescence lines are observed in confocal microscopy. These lines behave very much as single excitons in quantum dots, but their implementation is by far much easier, since it does not require 3D nucleation. The photon antibunching is demonstrated by time resolved Hanbury Brown and Twiss measurements.
Dibenzo[hi,st]ovalene as Highly Luminescent Nanographene: Efficient Synthesis via Photochemical Cyclodehydroiodination, Optoelectronic Properties, an…
2019
Dibenzo[hi,st]ovalene (DBOV), as a new nanographene, has demonstrated promising optical properties, such as red emission with a high fluorescence quantum yield of 79% and stimulated emission, as well as high thermal stability and photostability, which indicated its promise as a light-emitting and optical gain material. However, the previous synthetic routes required at least 12 steps. This obstructed access to different derivatives, e.g., to obtain crystals suitable for X-ray diffraction analysis and to tune the optoelectronic properties. Here, we report an efficient synthetic pathway to DBOV based on a sequential iodination-benzannulation of bi(naphthylphenyl)diyne, followed by photochemic…
Collective atomic effects in resonance fluorescence
1977
We suggest that the statistical properties of the scattered radiation in resonance-fluorescence experiments may be affected significantly by the existence of atomic correlations. The scattered light spectrum from two- and three-atom collective systems has been calculated and compared with the one-atom spectrum. The differences are quite significant for weak fields, but become less pronounced as the intensity of the driving field is increased. In addition, we have calculated the scattered intensity correlation function for collectively interacting systems, and found that its behavior is very different from that of the single-atom intensity correlation function, both for weak and strong incid…
Enhancement of thermal photon production in event-by-event hydrodynamics
2011
Thermal photon emission is widely believed to reflect properties of the earliest, hottest evolution stage of the medium created in ultra-relativistic heavy-ion collisions. Previous computations of photon emission have been carried out using a hydrodynamical medium description with smooth, averaged initial conditions. Recently, more sophisticated hydrodynamical models which calculate observables by averaging over many evolutions with event-by-event fluctuating initial conditions (IC) have been developed. Given their direct connection to the early time dynamics, thermal photon emission appears an ideal observable to probe fluctuations in the medium initial state. In this work, we demonstrate …
Photon antibunching and collective effects in the fluorescence of single bichromophoric molecules.
2003
The fluorescence of individual pairs of perylenemonoimide chromophores coupled via a short rigid linker is investigated. Photon antibunching is reported, indicating collective effects in the fluorescence, which are further substantiated by the observation of collective triplet off times and triplet lifetime shortening. The experimental findings are analyzed in terms of singlet-singlet and singlet-triplet annihilation based on Forster type energy transfer. The results reported here demonstrate that the statistical properties of the emission light of isolated single quantum systems can serve as a hallmark of intermolecular interactions.